Citation:
Juanjuan Shi, Renfeng Nie, Mengyuan Zhang, Mengsi Zhao, Zhaoyin Hou. Microwave-assisted fast fabrication of a nanosized Pt3Co alloy on reduced graphene oxides[J]. Chinese Journal of Catalysis,
;2014, 35(12): 2029-2037.
doi:
10.1016/S1872-2067(14)60232-1
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Ultrafine and homogenously dispersed Pt3Co alloy nanoparticles were fabricated on reduced graphene oxide (RGO) in a few minutes under microwave irradiation. Characterization results confirmed that microwave irradiation was important for higher metal utilization, the easy control of alloy composition, improved dispersion of the Pt3Co particles and minimizing the re-graphitization of the parent RGO by comparison with conventional solvent-thermal and impregnation methods. This Pt3Co/RGO-MW catalyst was extremely active and selective during the hydrogenation of cinnamaldehyde to cinnamyl alcohol. The calculated specific activity of each Pt atom in the Pt3Co/RGO-MW at 70 ℃ was 23.8 min-1.
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Keywords:
- graphene,
- Pt3Co,
- microwave irradiation,
- cinnamaldehyde,
- hydrogenation
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[1]
[1] Tian N, Zhou Z Y, Sun S G, Ding Y, Wang Z L. Science, 2007, 316: 732
-
[2]
[2] Stamenkovic V R, Mun B S, Arenz M, Mayrhofer K J J, Lucas C A, Wang G F, Ross P N, Markovic N M. Nat Mater, 2007, 6: 241
-
[3]
[3] Ghosh T, Leonard B M, Zhou Q, DiSalvo F J. Chem Mater, 2010, 22: 2190
-
[4]
[4] Jusys Z, Behm R J. J Phys Chem B, 2001, 105: 10874
-
[5]
[5] Lee A F, Gee J J, Theyers H J. Green Chem, 2000, 2: 279
-
[6]
[6] Nie R F, Liang D, Shen L, Gao J, Chen P, Hou Z Y. Appl Catal B, 2012, 127: 212
-
[7]
[7] Liang D, Gao J, Sun H, Chen P, Hou Z Y, Zheng X M. Appl Catal B, 2011, 106: 423
-
[8]
[8] Tsang S C, Cailuo N, Oduro W, Kong A T S, Clifton L, Yu K M K, Thiebaut B, Cookson J, Bishop P. ACS Nano, 2008, 2: 2547
-
[9]
[9] Shi J J, Nie R F, Chen P, Hou Z Y. Catal Commun, 2013, 41: 101
-
[10]
[10] Vu H, Gonçalves F, Philippe R, Lamouroux E, Corrias M, Kihn Y, Plee D, Kalck P, Serp P. J Catal, 2006, 240: 18
-
[11]
[11] Yang H Z, Zhang J, Sun K, Zou S Z, Fang J Y. Angew Chem Int Ed, 2010, 49: 6848
-
[12]
[12] Choi S I, Choi R, Han S W, Park J T. Chem-Eur J, 2011, 17: 12280
-
[13]
[13] Wang C, Wang G F, van der Vliet D, Chang K C, Markovic N M, Stamenkovic V R. Phys Chem Chem Phys, 2010, 12: 6933
-
[14]
[14] Callejas-Tovar R, Liao W T, de la Hoz J M M, Balbuena P B. J Phys Chem C, 2011, 115: 4104
-
[15]
[15] Wu B H, Huang H Q, Yang J, Zheng N F, Fu G. Angew Chem Int Ed, 2012, 51: 3440
-
[16]
[16] Kwon S G, Krylova G, Sumer A, Schwartz M M, Bunel E E, Marshall C L, Chattopadhyay S, Lee B, Jellinek J, Shevchenko E V. Nano Lett, 2012, 12: 5382
-
[17]
[17] Shao Y Y, Zhang S, Wang C M, Nie Z M, Liu J, Wang Y, Lin Y H. J Power Sources, 2010, 195: 4600
-
[18]
[18] Guo S J, Dong S J, Wang E K. ACS Nano, 2010, 4: 547
-
[19]
[19] Kundu P, Nethravathi C, Deshpande P A, Rajamathi M, Madras G, Ravishankar N. Chem Mater, 2011, 23: 2772
-
[20]
[20] Bock C, Paquet C, Couillard M, Botton G A, MacDougall B R. J Am Chem Soc, 2004,126: 8028
-
[21]
[21] Santori G F, Casella M L, Ferretti O A. J Mol Catal A, 2002, 186: 223
-
[22]
[22] Yue Q L, Zhang K, Chen X M, Wang L, Zhao J S, Liu J F, Jia J B. Chem Commun, 2010, 46: 3369
-
[23]
[23] Scheuermann G M, Rumi L, Steurer P, Bannwarth W, Mülhaupt R. J Am Chem Soc, 2009, 131: 8262
-
[24]
[24] Nie R F, Wang J H, Wang L N, Qin Y, Chen P, Hou Z Y. Carbon, 2012, 50: 586
-
[25]
[25] Siamaki A R, Khder A E R S, Abdelsayed V, El-Shall M S, Gupton B F. J Catal, 2011, 279: 1
-
[26]
[26] Zhao Y C, Zhan L, Tian J N, Nie S L, Ning Z. Electrochim Acta, 2011, 56: 1967
-
[27]
[27] Verma S, Mungse H P, Kumar N, Choudhary S, Jain S L, Sain B, Khatri O P. Chem Commun, 2011, 47: 12673
-
[28]
[28] Allen M J, Tung V C, Kaner R B. Chem Rev, 2010, 110: 132
-
[29]
[29] Si Y C, Samulski E T. Chem Mater, 2008, 20: 6792
-
[30]
[30] Chen S Q, Wang Y. J Mater Chem, 2010, 20: 9735
-
[31]
[31] Hu H, Zhao Z B, Zhou Q, Gogotsi Y, Qiu J S. Carbon, 2012, 50: 3267
-
[32]
[32] Knupp S L, Li W Z, Paschos O, Murray T M, Snyder J, Haldar P. Carbon, 2008, 46: 1276
-
[33]
[33] Jiang S J, Ma Y W, Jian G Q, Tao H S, Wang X Z, Fan Y N, Lu Y N, Hu Z, Chen Y. Adv Mater, 2009, 21: 4953
-
[34]
[34] Yu W Y, Tu W X, Liu H F. Langmuir, 1999, 15: 6
-
[35]
[35] Hummers W S Jr, Offemann R E. J Am Chem Soc, 1958, 80: 1339
-
[36]
[36] Fei L F, Sun T Y, Lu W, An X Q, Hu Z F, Yu J C, Zheng R K, Li X M, Chan H L W, Wang Y. Chem Commun, 2014, 50: 826
-
[37]
[37] Li X L, Zhang G Y, Bai X D, Sun X M, Wang X R, Wang E G, Dai H J. Nat Nanotechnol, 2008, 3: 538
-
[38]
[38] Chen J L, Yan X P. J Mater Chem, 2010, 20: 4328
-
[39]
[39] Pimenta M A, Dresselhaus G, Dresselhaus M S, Cançado L G, Jorio A, Saito R. Phys Chem Chem Phys, 2007, 9: 1276
-
[40]
[40] Paredes J I, Villar-Rodil S, Solís-Fernández P, Martínez-Alonso A, Tascón J M D. Langmuir, 2009, 25: 5957
-
[41]
[41] Vinayan B P, Ramaprabhu S. Nanoscale, 2013, 5: 5109
-
[42]
[42] Liang Y M, Zhang H M, Zhong H X, Zhu X B, Tian Z Q, Xu D Y, Yi B L. J Catal, 2006, 238: 468
-
[43]
[43] Gao C L, Liang Y Y, Han M, Xu Z, Zhu J M. J Phys Chem C, 2008, 112: 9272
-
[44]
[44] Duong H T, Rigsby M A, Zhou W P, Wieckowski A. J Phys Chem C, 2007, 111: 13460
-
[45]
[45] Li Y, Zhu P F, Zhou R X. Appl Surf Sci, 2008, 254: 2609
-
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