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Citation: Lei Pang, Chi Fan, Lina Shao, Junxia Yi, Xing Cai, Jian Wang, Ming Kang, Tao Li. Effect of V2O5/WO3-TiO2 catalyst preparation method on NOx removal from diesel exhaust[J]. Chinese Journal of Catalysis, ;2014, 35(12): 2020-2028. doi: 10.1016/S1872-2067(14)60218-7 shu

Effect of V2O5/WO3-TiO2 catalyst preparation method on NOx removal from diesel exhaust

  • 1.

    a. School of Chemistry & Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei, China;

  • Corresponding author: Tao Li, 
  • Received Date: 20 June 2014
    Available Online: 2 September 2014

  • V2O5/WO3-TiO2 catalysts were prepared by conventional impregnation (VWTi-con) and ultras­ound-assisted impregnation methods (VWTi-HUST). Their catalytic performance was tested for the selective catalytic reduction (SCR) of NO with NH3. The effects of the preparation methods on the catalyst properties were studied. The catalysts were characterized by X-ray diffraction, scanning electron microscopy, Raman and X-ray photoelectron spectroscopy. Both structural investigation and NH3-SCR activity showed that the preparation method had a strong effect on the thermal behavior of the V2O5/WO3-TiO2 catalysts. After a hydrothermal treatment, a significant loss of NO reduction activity was observed for the VWTi-con catalyst, which suffered severe sintering and even formed a rutile VxTi1-xO2 solid solution, while the VWTi-HUST catalyst had the same good hydrothermal stability as a commercial catalyst, indicating that the VWTi-HUST catalyst can be used in a commercial diesel after-treatment system. The ultrasound-assisted impregnation method produced a stronger interaction between the vanadium species and WTi support, which stabilized the vanadium species in the reduced state.
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    1. [1]

      [1] Kašpar J, Fornasiero P, Hickey N. Catal Today, 2003, 77: 419

    2. [2]

      [2] Schultz M G, Diehl T, Brasseur G P, Zittel W. Science, 2003, 302: 624

    3. [3]

      [3] Skalska K, Miller J S, Ledakowicz S. Sci Total Environ, 2010, 408: 3976

    4. [4]

      [4] Nakajima F, Hamada I. Catal Today, 1996, 29: 109

    5. [5]

      [5] Forzatti P. Appl Catal A, 2001, 222: 221

    6. [6]

      [6] Liu Z M, Woo S I. Catal Rev-Sci Eng, 2006, 48: 43

    7. [7]

      [7] Liu F D, Shan W P, Shi X Y, He H. Chem Prog (刘福东, 单文坡, 石晓燕, 贺泓. 化学进展), 2012, 24: 446

    8. [8]

      [8] Zhao Z, Zhang G Z, Liu J, Liang P, Xu J, Duan A J, Jiang G Y, Xu C M. Chin J Catal (赵震, 张桂臻, 刘坚, 梁鹏, 许洁, 段爱军, 姜桂元, 徐春明. 催化学报), 2008, 29: 303

    9. [9]

      [9] Li J H, Chang H Z, Ma L, Hao J M, Yang R T. Catal Today, 2011, 175: 147

    10. [10]

      [10] Kobayashi M, Kuma R, Masaki S, Sugishima N. Appl Catal B, 2005, 60: 173

    11. [11]

      [11] Kröcher O, Elsener M. Appl Catal B, 2008, 77: 215

    12. [12]

      [12] Choo S T, Lee Y G, Nam I S, Ham S W, Lee J B. Appl Catal A, 2000, 200: 177

    13. [13]

      [13] Li M, Altman E I. J Phys Chem C, 2009, 113: 2798

    14. [14]

      [14] Wachs I E. J Catal, 1990, 124: 570

    15. [15]

      [15] Tang F S, Zhuang K, Yang F, Yang L L, Xu B L, Qiu J H, Fan Y N. Chin J Catal (唐富顺, 庄柯, 杨芳, 杨利利, 许波连, 邱金恒, 范以宁. 催化学报), 2012, 33: 933

    16. [16]

      [16] Wachs I E, Weckhuysen B M. Appl Catal A, 1997, 157: 67

    17. [17]

      [17] Xu H D, Fang Z T, Cao Y, Kong S, Lin T, Gong M C, Chen Y Q. Chin J catal (徐海迪, 房志涛, 曹毅, 孔爽, 林涛, 龚茂初, 陈耀强. 催化学报), 2012, 33: 1927

    18. [18]

      [18] Odenbrand C U I. Chem Eng Res Des, 2008, 86: 663

    19. [19]

      [19] Madia G, Elsener M, Koebel M, Raimondi F, Wokaun A. Appl Catal B, 2002, 39: 181

    20. [20]

      [20] Van Setten B A A L, Makkee M, Moulijn J A. Catal Rev-Sci Eng, 2001, 43: 489

    21. [21]

      [21] Thiruvengadam A, Besch M C, Carder D K, Oshinuga A, Gautam M. Environ Sci Technol, 2012, 46: 1907

    22. [22]

      [22] Reddy B M, Mehdi S, Reddy E P. Catal Lett, 1993, 20: 317

    23. [23]

      [23] Albonetti S, Blasioli S, Bugani M, Lehaut-Burnouf C, Augustine S, Roncari E, Trifirò F. Environ Chem Lett, 2003, 1: 197

    24. [24]

      [24] Reddy B M, Kumar M V, Reddy E P, Mehdi S. Catal Lett, 1996, 36: 187

    25. [25]

      [25] Shi A J, Wang X Q, Yu T, Shen M Q. Appl Catal B, 2011, 106: 359

    26. [26]

      [26] Casanova M, Schermanz K, Llorca J, Trovarelli A. Catal Today, 2012, 184: 227

    27. [27]

      [27] Reiche M A, Hug P, Baiker A. J Catal, 2000, 192: 400

    28. [28]

      [28] Reddy B M, Ganesh I, Reddy E P. J Phys Chem B, 1997, 101: 1769

    29. [29]

      [29] Chiker F, Nogier J P, Bonardet J L. Catal Today, 2003, 78: 139

    30. [30]

      [30] Went G T, Leu L, Bell A T. J Catal, 1992, 134: 479

    31. [31]

      [31] Yu X F, Wu N Z, Xie Y C, Tang Y Q. J Mater Sci Lett, 2001, 20: 319

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