Citation: Zi-Guang Zhao, Yi-Chao Xu, Ruo-Chen Fang, Ming-Jie Liu. Bioinspired Adaptive Gel Materials with Synergistic Heterostructures[J]. Chinese Journal of Polymer Science, ;2018, 36(6): 683-696. doi: 10.1007/s10118-018-2105-z shu

Bioinspired Adaptive Gel Materials with Synergistic Heterostructures

a.
Key Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, China
b.
International Research Institute for Multidisciplinary Science, Beihang University, Beijing 100191, China
c.
Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, China

Corresponding author: Ming-Jie Liu, liumj@buaa.edu.cn
Received Date: 22 November 2017
Accepted Date: 22 December 2017
Available Online: 8 February 2018

In nature, many biological soft tissues with synergistic heterostructures, such as sea cucumbers, skeletal muscles and cartilages, exhibit high functionality to adapt to complex environments. In artificial soft materials, hydrogels are similar to biological soft tissues due to the unique integration of "soft and wet" properties and elastic characteristics. However, currently hydrogel materials lack their necessary adaptability, including narrow working temperature windows and uncontrollable mechanics, thus restrict their engineering application in complex environments. Inspired by abovementioned biological soft tissues, researchers have increasingly developed heterostructural gel materials as functional soft materials with high adaptability to various mechanical and environmental conditions. This article summarizes our recent work on high-performance adaptive gel materials with synergistic heterostructures, including the critical design criteria and the state-of-the-art fabrication strategies of our gel materials. The functional adaptation properties of these heterostructural gel materials are also presented in details, including temperature, wettability, mechanical and shape adaption.
- Bioinspired materials,
- Adaptive gels,
- Hydrogels,
- Mechanical strength,
- Shape memory
1. [1]
  Zhao Z., Fang R., Rong Q., Liu M.. Bioinspired nanocomposite hydrogels with highly ordered structures[J]. Adv. Mater., 2017,29(45). doi: 10.1002/adma.201703045
2. [2]
  Slaughter B. V., Khurshid S. S., Fisher O. Z., Khademhosseini A., Peppas N. A.. Hydrogels in regenerative medicine[J]. Adv. Mater., 2009,21(32):3307-3329.
3. [3]
  Liu M., Wang S., Jiang L.. Nature-inspired superwettability systems[J]. Nat. Rev. Mater., 2017,217036. doi: 10.1038/natrevmats.2017.36
4. [4]
  Chen L., Yin Y., Liu Y., Lin L., Liu M.. Design and fabrication of functional hydrogels through interfacial engineering[J]. Chinese J. Polym. Sci., 2017,35(10):1181-1193. doi: 10.1007/s10118-017-1995-5
5. [5]
  Lee K. Y., Mooney D. J.. Hydrogels for tissue engineering[J]. Chem. Rev., 2001,101(7):1869-1880. doi: 10.1021/cr000108x
6. [6]
  Taylor D. L., Panhuis M.. Self-healing hydrogels[J]. Adv. Mater., 2016,28(41):9060-9093. doi: 10.1002/adma.201601613
7. [7]
  Yuk H., Lin S., Ma C., Takaffoli M., Fang N. X., Zhao X.. Hydraulic hydrogel actuators and robots optically and sonically camouflaged in water[J]. Nat. Commun., 2017,8. doi: 10.1038/ncomms14230
8. [8]
  Lee B. P., Konst S.. Novel hydrogel actuator inspired by reversible mussel adhesive protein chemistry[J]. Adv. Mater., 2014,26(21):3415-3419. doi: 10.1002/adma.v26.21
9. [9]
  Shin M. K., Spinks G. M., Shin S. R., Kim S. I., Kim S. J.. Nanocomposite hydrogel with high toughness for bioactuators[J]. Adv. Mater., 2009,21(17):1712-1715. doi: 10.1002/adma.v21:17
10. [10]
  Shin S. R., Jung S. M., Zalabany M., Kim K., Zorlutuna P., Kim S. B., Nikkhah M., Khabiry M., Azize M., Kong J., Wan K. T., Palacios T., Dokmeci M. R., Bae H., Tang X., Khademhosseini A.. Carbon-nanotube-embedded hydrogel sheets for engineering cardiac constructs and bioactuators[J]. ACS Nano, 2013,7(3):2369-2380. doi: 10.1021/nn305559j
11. [11]
  Culver H. R., Clegg J. R., Peppas N. A.. Analyte-responsive hydrogels:intelligent materials for biosensing and drug delivery[J]. Acc. Chem. Res., 2017,50(2):170-178. doi: 10.1021/acs.accounts.6b00533
12. [12]
  Xing J. F., Zheng M. L., Duan X. M.. Two-photon polymerization microfabrication of hydrogels:an advanced 3D printing technology for tissue engineering and drug delivery[J]. Chem. Soc. Rev., 2015,44:5031-5039. doi: 10.1039/C5CS00278H
13. [13]
  Wang P., Sun J., Lou Z., Fan F., Hu K., Sun Y., Gu N.. Assembly-induced thermogenesis of gold nanoparticles in the presence of alternating magnetic field for controllable drug release of hydrogel[J]. Adv. Mater., 2016,28(48):10801-10808. doi: 10.1002/adma.201603632
14. [14]
  Liu J., Tan C. S., Yu Z., Lan Y., Abell C., Scherman O. A.. Biomimetic supramolecular polymer networks exhibiting both toughness and self-recovery[J]. Adv. Mater., 2017,29(10). doi: 10.1002/adma.201604951
15. [15]
  Liu Z., Calvert P.. Multilayer hydrogels as muscle-like actuators[J]. Adv. Mater., 2000,12(4):288-291. doi: 10.1002/(ISSN)1521-4095
16. [16]
  VanBemmelen J. M.. Der hydrogel und das kristallinische hydrat des kupferoxydes[J]. Z. Anorg. Chem., 1894,5:466-483. doi: 10.1002/(ISSN)1521-3749
17. [17]
  Wichterle O., Lím D.. Hydrophilic gels for biological use[J]. Nature, 1960,185:117-118. doi: 10.1038/185117a0
18. [18]
  Jokl J., Kopeček J., Lím D.. Mechanism of three-dimensional polymerization of the system methyl methacrylate-glycol dimethacrylate.Ⅰ. Determination of the structure of the threedimensional product[J]. J. Polym. Sci. A1 Polym. Chem., 1968,6(11):3041-3048. doi: 10.1002/pol.1968.150061108
19. [19]
  Refojo M. F., Yasuda H.. Hydrogels from 2-hydroxyethyl methacrylate and propylene glycol monoacrylate[J]. J. Appl. Polym. Sci., 1965,9(7):2425-2435. doi: 10.1002/app.1965.070090707
20. [20]
  Hicks G. P., Updike S. J.. The preparation and characterization of lyophilized polyacrylamide enzyme gels for chemical analysis[J]. Anal. Chem., 1966,38(6):726-730. doi: 10.1021/ac60238a014
21. [21]
  Freeman A., Aharonowitz Y.. Immobilization of microbial cells in crosslinked, prepolymerized, linear polyacrylamide gels:antibiotic production by immobilized Streptomyces clavuligerus cells[J]. Biotechnol. Bioeng., 1981,23(12):2747-2759. doi: 10.1002/(ISSN)1097-0290
22. [22]
  Otake K., Inomata H., Konno M., Saito S.. Thermal analysis of the volume phase transition with N-isopropylacrylamide gels[J]. Macromolecules, 1990,23(1):283-289. doi: 10.1021/ma00203a049
23. [23]
  Inomata H., Goto S., Saito S.. Phase transition of N-substituted acrylamide gels[J]. Macromolecules, 1990,23(22):4887-4888. doi: 10.1021/ma00224a023
24. [24]
  Dong L. C., Qi Y., Hoffman A. S.. Controlled release of amylase from a thermal and pH-sensitive, macroporous hydrogel[J]. J. Control. Release, 1992,19(1):171-177.
25. [25]
  Zhao X.. Multi-scale multi-mechanism design of tough hydrogels:building dissipation into stretchy networks[J]. Soft Matter, 2014,10:672-687. doi: 10.1039/C3SM52272E
26. [26]
  Haraguchi K., Takehisa T., Ebato M.. Control of cell cultivation and cell sheet detachment on the surface of polymer/clay nanocomposite hydrogels[J]. Biomacromolecules, 2006,7(11):3267-3275. doi: 10.1021/bm060549b
27. [27]
  Haraguchi K., Li H. J.. Control of the coil-to-globule transition and ultrahigh mechanical properties of PNIPA in nanocomposite hydrogels[J]. Angew. Chem. Int. Ed., 2005,44(40):6500-6504. doi: 10.1002/(ISSN)1521-3773
28. [28]
  Gong J. P., Katsuyama Y., Kurokawa T., Osada Y.. Doublenetwork hydrogels with extremely high mechanical strength[J]. Adv. Mater., 2003,15(14):1155-1158. doi: 10.1002/adma.200304907
29. [29]
  Sun J. Y., Zhao X., Illeperuma W. R., Chaudhuri O., Oh K. H., Mooney D. J., Vlassak J. J., Suo Z.. Highly stretchable and tough hydrogels[J]. Nature, 2012,489:133-136. doi: 10.1038/nature11409
30. [30]
  Rauner N., Meuris M., Zoric M., Tiller J. C.. Enzymatic mineralization generates ultrastiff and tough hydrogels with tunable mechanics[J]. Nature, 2017,543:407-410. doi: 10.1038/nature21392
31. [31]
  Wang Q., Mynar J. L., Yoshida M., Lee E., Lee M., Okuro K., Kinbara K., Aida T.. High-water-content mouldable hydrogels by mixing clay and a dendritic molecular binder[J]. Nature, 2010,463:339-343. doi: 10.1038/nature08693
32. [32]
  Kamata H., Akagi Y., Kayasuga-Kariya Y., Chung U. I., Sakai T.. "Nonswellable" hydrogel without mechanical hysteresis[J]. Science, 2014,343(6173):873-875. doi: 10.1126/science.1247811
33. [33]
  Liu M., Ishida Y., Ebina Y., Sasaki T., Hikima T., Takata M., Aida T.. An anisotropic hydrogel with electrostatic repulsion between cofacially aligned nanosheets[J]. Nature, 2015,517:68-72. doi: 10.1038/nature14060
34. [34]
  Kim H. N., Jiao A., Hwang N. S., Kim M. S., Kang D. H., Kim D. H., Suh K. Y.. Nanotopography-guided tissue engineering and regenerative medicine[J]. Adv. Drug. Delivery Rev., 2013,65(4):536-558. doi: 10.1016/j.addr.2012.07.014
35. [35]
  Liu M., Jiang L.. Dialectics of nature in materials science:binary cooperative complementary materials[J]. Sci. China Mater., 2016,59(4):239-246. doi: 10.1007/s40843-016-5051-6
36. [36]
  Oliva N., Conde J., Wang K., Artzi N.. Designing hydrogels for on-demand therapy[J]. Acc. Chem. Res., 2017,50(4):669-679. doi: 10.1021/acs.accounts.6b00536
37. [37]
  Dou X. Q., Feng C. L.. Amino acids and peptide-based supramolecular hydrogels for three-dimensional cell culture[J]. Adv. Mater., 2017,29(16)1604062. doi: 10.1002/adma.201604062
38. [38]
  Wegst U. G., Bai H., Saiz E., Tomsia A. P., Ritchie R. O.. Bioinspired structural materials[J]. Nat. Mater., 2015,14:23-36. doi: 10.1038/nmat4089
39. [39]
  Motokawa T.. Effects of ionic environment on viscosity of Triton-extracted catch connective tissue of a sea cucumber body wall[J]. Comp. Biochem. Physiol. Part B, 1994,109(4):613-622. doi: 10.1016/0305-0491(94)90124-4
40. [40]
  Thurmond F. A., Trotter J. A.. Morphology and biomechanics of the microfibrillar network of sea cucumber dermis[J]. J. Exp. Biol., 1996,199:1817-1828.
41. [41]
  Szulgit G. K., Shadwick R. E.. Dynamic mechanical characterization of a mutable collagenous tissue:response of sea cucumber dermis to cell lysis and dermal extracts[J]. J. Exp. Biol., 2000,203(10):1539-1550.
42. [42]
  Capadona J. R., Shanmuganathan K., Tyler D. J., Rowan S. J., Weder C.. Stimuli-responsive polymer nanocomposites inspired by the sea cucumber dermis[J]. Science, 2008,319(5868):1370-1374. doi: 10.1126/science.1153307
43. [43]
  Mo J., Prévost S. F., Blowes L. M., Egertová M., Terrill N. J., Wang W., Elphick M. R., Gupta H. S.. Interfibrillar stiffening of echinoderm mutable collagenous tissue demonstrated at the nanoscale[J]. P. Natl. Acad. Sci. USA, 2016,113(42):E6362-E6371. doi: 10.1073/pnas.1609341113
44. [44]
  Johnson M. A., Polgar J., Weightman D., Appleton D.. Data on the distribution of fibre types in thirty-six human muscles:an autopsy study[J]. J. Neurol. Sci., 1973,18(1):111-129. doi: 10.1016/0022-510X(73)90023-3
45. [45]
  Tiidus, P. M., "Skeletal muscle damage and repair", Human Kinetics Press, Champaign, IL USA, 2008, p. 37
46. [46]
  Wakelam M. J.. The fusion of myoblasts[J]. Biochem. J., 1985,228:1-12. doi: 10.1042/bj2280001
47. [47]
  Wigmore P. M., Dunglison G. F.. The generation of fiber diversity during myogenesis[J]. Int. J. Dev. Biol., 1998,42(2):117-125.
48. [48]
  Jana S., Levengood S. K., Zhang M.. Anisotropic materials for skeletal-muscle-tissue engineering[J]. Adv. Mater., 2016,28(48):10588-10612. doi: 10.1002/adma.201600240
49. [49]
  Kerin A. J., Wisnom M. R., Adams M. A.. The compressive strength of articular cartilage[J]. Proc. Inst. Mech. Eng. Part H, 1998,212(4):273-280. doi: 10.1243/0954411981534051
50. [50]
  Tepic S., Macirowski T., Mann R. W.. Mechanical properties of articular cartilage elucidated by osmotic loading and ultrasound[J]. Proc. Natl. Acad. Sci. USA, 1983,80(11):3331-3333. doi: 10.1073/pnas.80.11.3331
51. [51]
  Fratzl P., Weinkamer R.. Nature's hierarchical materials[J]. Prog. Mater. Sci., 2007,52(8):1263-1334. doi: 10.1016/j.pmatsci.2007.06.001
52. [52]
  Simha N. K., Carlson C. S., Lewis J. L.. Evaluation of fracture toughness of cartilage by micropenetration[J]. J. Mater. Sci. Mater. Med., 2004,15(5):631-639. doi: 10.1023/B:JMSM.0000026104.30607.c7
53. [53]
  Ker R. F.. The design of soft collagenous load-bearing tissues[J]. J. Exp. Biol., 1999,202(23):3315-3324.
54. [54]
  Bellucci G., Seedhom B. B.. Mechanical behaviour of articular cartilage under tensile cyclic load[J]. Rheumatology, 2001,40(12):1337-1345. doi: 10.1093/rheumatology/40.12.1337
55. [55]
  Salt R. W.. Survival of frozen fat body cells in an insect[J]. Nature, 1959,184:1426-1426.
56. [56]
  Thomashow M. F.. Plant cold acclimation:freezing tolerance genes and regulatory mechanisms[J]. Annu. Rev. Plant Physiol. Plant Mol. Biol., 1999,50:571-599. doi: 10.1146/annurev.arplant.50.1.571
57. [57]
  Moellering E. R., Muthan B., Benning C.. Freezing tolerance in plants requires lipid remodeling at the outer chloroplast membrane[J]. Science, 2010,330(6001):226-228. doi: 10.1126/science.1191803
58. [58]
  Takahashi D., Imai H., Kawamura Y., Uemura M.. Lipid profiles of detergent resistant fractions of the plasma membrane in oat and rye in association with cold acclimation and freezing tolerance[J]. Cryobiology, 2016,72(2):123-134. doi: 10.1016/j.cryobiol.2016.02.003
59. [59]
  Martz F., Sutinen M. L., Kiviniemi S., Palta J. P.. Changes in freezing tolerance, plasma membrane H+-ATPase activity and fatty acid composition in Pinus resinosa needles during cold acclimation and de-acclimatio[J]. Tree Physiol., 2006,26(6):783-790. doi: 10.1093/treephys/26.6.783
60. [60]
  Gao H., Zhao Z., Cai Y., Zhou J., Hua W., Chen L., Wang L., Zhang J., Han D., Liu M., Jiang L.. Adaptive and freezetolerant heteronetwork organohydrogels with enhanced mechanical stability over a wide temperature range[J]. Nat. Commun., 2017,8. doi: 10.1038/ncomms15911
61. [61]
  Rong Q., Lei W., Chen L., Yin Y., Zhou J., Liu M.. Antifreezing, conductive self-healing organohydrogels with stable strain-sensitivity at subzero temperatures[J]. Angew. Chem. Int. Ed., 2017,129(45):14347-14351. doi: 10.1002/ange.201708614
62. [62]
  Shi S., Peng X., Liu T., Chen Y. N., He C., Wang H.. Facile preparation of hydrogen-bonded supramolecular polyvinyl alcohol-glycerol gels with excellent thermoplasticity and mechanical properties[J]. Polymer, 2017,111(24):168-176.
63. [63]
  Shin J., Lee J. S., Lee C., Park H. J., Yang K., Jin Y., Ryu J. H., Hong K. S., Moon S. H., Chung H. M., Yang H. S., Um S. H., Oh J. W., Kim D. I., Lee H., Cho S. W.. Tissue adhesive catechol-modified hyaluronic acid hydrogel for effective, minimally invasive cell therapy[J]. Adv. Funct. Mater., 2015,25(25):3814-3824. doi: 10.1002/adfm.v25.25
64. [64]
  Liu Y., Meng H., Konst S., Sarmiento R., Rajachar R., Lee B. P.. Injectable dopamine-modified poly(ethylene glycol) nanocomposite hydrogel with enhanced adhesive property and bioactivity[J]. ACS Appl. Mater. Interfaces, 2014,6(19):16982-16992. doi: 10.1021/am504566v
65. [65]
  Lee Y. B., Shin Y. M., Kim E. M., Lim J., Lee J. Y., Shin H.. Facile cell sheet harvest and translocation mediated by a thermally expandable hydrogel with controlled cell adhesion[J]. Adv. Healthc. Mater., 2016,5(18):2320-2324. doi: 10.1002/adhm.v5.18
66. [66]
  Thornton D. J., Sheehan J. K.. From mucins to mucus:toward a more coherent understanding of this essential barrier[J]. Proc. Am. Thorac. Soc., 2004,1(1):54-61. doi: 10.1513/pats.2306016
67. [67]
  Weis K.. The nuclear pore complex:oily spaghetti or gummy bear?[J]. Cell, 2007,130(3):405-407. doi: 10.1016/j.cell.2007.07.029
68. [68]
  Yao X., Chen L., Ju J., Li C., Tian Y., Jiang L., Liu M.. Superhydrophobic diffusion barriers for hydrogels via confined interfacial modification[J]. Adv. Mater., 2016,28(34):7383-7389. doi: 10.1002/adma.201601568
69. [69]
  Chen L., Yao X., Gu Z., Zheng K., Zhao C., Lei W., Rong Q., Lin L., Wang J., Jiang L., Liu M.. Covalent tethering of photo-responsive superficial layers on hydrogel surfaces for photo-controlled release[J]. Chem. Sci., 2017,8:2010-2016. doi: 10.1039/C6SC04634G
70. [70]
  Chen H., Yang F. Y., Chen Q., Zheng J.. A novel design of multi-mechanoresponsive and mechanically strong hydrogels[J]. Adv. Mater., 2017,29(21). doi: 10.1002/adma.201606900
71. [71]
  Bilici C., Can V., Nçchel U., Behl M., Lendlein A., Okay O.. Melt-processable shape-memory hydrogels with self-healing ability of high mechanical strength[J]. Macromolecules, 2016,49(19):7442-7449. doi: 10.1021/acs.macromol.6b01539
72. [72]
  Luo R. C., Wu J., Dinh N. D., Chen C. H.. Gradient porous elastic hydrogels with shape-memory property and anisotropic responses for programmable locomotion[J]. Adv. Funct. Mater., 2015,25(47):7272-7279. doi: 10.1002/adfm.v25.47
73. [73]
  Wang W., Zhang Y. Y., Liu W. G.. Bioinspired fabrication of high strength hydrogels from non-covalent interactions[J]. Prog. Polym. Sci., 2017,71:1-25. doi: 10.1016/j.progpolymsci.2017.04.001
74. [74]
  Dai X. Y., Zhang Y. Y., Gao L. N., Bai T., Wang W., Cui Y. L., Liu W. G.. A mechanically strong, highly stable, thermoplastic, and self-healable supramolecular polymer hydrogel[J]. Adv. Mater., 2015,27(23):3566-3571. doi: 10.1002/adma.v27.23
75. [75]
  Lu C. H., Guo W., Hu Y., Qi X. J., Willner I.. Multitriggered shape-memory acrylamide-DNA hydrogels[J]. J. Am. Chem. Soc., 2015,137(50):15723-15731. doi: 10.1021/jacs.5b06510
76. [76]
  Zhao Z., Zhang K., Liu Y., Zhou J., Liu M.. Highly stretchable, shape memory organohydrogels using phasetransition microinclusions[J]. Adv. Mater., 2017,29(33)1701695. doi: 10.1002/adma.v29.33
77. [77]
  Zhao Z., Liu Y., Zhang K., Zhuo S., Fang R., Zhang J., Jiang L., Liu M.. Biphasic synergistic gel materials with switchable mechanics and self-healing capacity[J]. Angew. Chem. Int. Ed., 2017,129(43):13649-13654. doi: 10.1002/ange.201707239
78. [78]
  Kim Y. S., Liu M., Ishida Y., Ebina Y., Osada M., Sasaki T., Hikima T., Takata M., Aida T.. Thermoresponsive actuation enabled by permittivity switching in an electrostatically anisotropic hydrogel[J]. Nat. Mater., 2015,14:1002-1007. doi: 10.1038/nmat4363
79. [79]
  Liu M., Ishida Y., Ebina Y., Sasaki T., Aida T.. Photolatently modulable hydrogels using unilamellar titania nanosheets as photocatalytic crosslinkers[J]. Nat. Commun., 2013,42029. doi: 10.1038/ncomms3029
1. [1]
  Jiajia Wang , XinXin Ge , Yajing Xiang , Xiaoliang Qi , Ying Li , Hangbin Xu , Erya Cai , Chaofan Zhang , Yulong Lan , Xiaojing Chen , Yizuo Shi , Zhangping Li , Jianliang Shen . An ionic liquid functionalized sericin hydrogel for drug-resistant bacteria-infected diabetic wound healing. Chinese Chemical Letters, 2025, 36(2): 109819-. doi: 10.1016/j.cclet.2024.109819
2. [2]
  Lijuan Liu , Xionglei Wang . Preparation of Hydrogels from Waste Thermosetting Unsaturated Polyester Resin by Controllable Catalytic Degradation: A Comprehensive Chemical Experiment. University Chemistry, 2024, 39(11): 313-318. doi: 10.12461/PKU.DXHX202403060
3. [3]
  Binhan Zhao , Zheng Li , Lan Zheng , Zhichao Ye , Yuyang Yuan , Shanshan Zhang , Bo Liang , Tianyu Li . Recent progress in the biomedical application of PEDOT:PSS hydrogels. Chinese Chemical Letters, 2024, 35(10): 109810-. doi: 10.1016/j.cclet.2024.109810
4. [4]
  Zikang Hu , Hengjie Zhang , Zhengqiu Li , Tianbao Zhao , Zhipeng Gu , Qijuan Yuan , Baoshu Chen . Multifunctional photothermal hydrogels: Design principles, various functions, and promising biological applications. Chinese Chemical Letters, 2024, 35(10): 109527-. doi: 10.1016/j.cclet.2024.109527
5. [5]
  Zhenhao Wang , Yuliang Tang , Ruyu Li , Shuai Tian , Yu Tang , Dehai Li . Bioinspired synthesis of cochlearol B and ganocin A. Chinese Chemical Letters, 2024, 35(7): 109247-. doi: 10.1016/j.cclet.2023.109247
6. [6]
  Zhe-Han Yang , Jie Yin , Lei Xin , Yuanfang Li , Yijie Huang , Ruo Yuan , Ying Zhuo . Research advancement of DNA-based intelligent hydrogels: Manufacture, characteristics, application of disease diagnosis and treatment. Chinese Chemical Letters, 2024, 35(10): 109558-. doi: 10.1016/j.cclet.2024.109558
7. [7]
  Yue Sun , Yingnan Zhu , Jiahang Si , Ruikang Zhang , Yalan Ji , Jinjie Fan , Yuze Dong . Glucose-activated nanozyme hydrogels for microenvironment modulation via cascade reaction in diabetic wound. Chinese Chemical Letters, 2025, 36(4): 110012-. doi: 10.1016/j.cclet.2024.110012
8. [8]
  Yanqiong Wang , Yaqi Hou , Fengwei Huo , Xu Hou . Fe³⁺ ion quantification with reusable bioinspired nanopores. Chinese Chemical Letters, 2025, 36(2): 110428-. doi: 10.1016/j.cclet.2024.110428
9. [9]
  Pei Cao , Yilan Wang , Lejian Yu , Miao Wang , Liming Zhao , Xu Hou . Dynamic asymmetric mechanical responsive carbon nanotube fiber for ionic logic gate. Chinese Chemical Letters, 2024, 35(6): 109421-. doi: 10.1016/j.cclet.2023.109421
10. [10]
  Yan Chen , Xinnan Wang , Yifan Lin , Chun Liu . Shape/dimension-controllable organic heterostructures from one monomer pair. Chinese Chemical Letters, 2025, 36(3): 109903-. doi: 10.1016/j.cclet.2024.109903
11. [11]
  Linshan Peng , Qihang Peng , Tianxiang Jin , Zhirong Liu , Yong Qian . Highly efficient capture of thorium ion by citric acid-modified chitosan gels from aqueous solution. Chinese Chemical Letters, 2024, 35(5): 108891-. doi: 10.1016/j.cclet.2023.108891
12. [12]
  Yanhua Peng , Xin Yu , Ting Wang . Adaptive nanoconfined Fenton-like reactions: Tailoring carbon pathways for sustainable water treatment and energy harvesting. Chinese Chemical Letters, 2024, 35(12): 110198-. doi: 10.1016/j.cclet.2024.110198
13. [13]
  Lian Sun , Honglei Wang , Ming Ma , Tingting Cao , Leilei Zhang , Xingui Zhou . Shape and composition evolution of Pt and Pt₃M nanocrystals under HCl chemical etching. Chinese Chemical Letters, 2024, 35(9): 109188-. doi: 10.1016/j.cclet.2023.109188
14. [14]
  Dongmei Yao , Junsheng Zheng , Liming Jin , Xiaomin Meng , Zize Zhan , Runlin Fan , Cong Feng , Pingwen Ming . Effect of surface oxidation on the interfacial and mechanical properties in graphite/epoxy composites composite bipolar plates. Chinese Chemical Letters, 2024, 35(11): 109382-. doi: 10.1016/j.cclet.2023.109382
15. [15]
  Manman Ou , Yunjian Zhu , Jiahao Liu , Zhaoxuan Liu , Jianjun Wang , Jun Sun , Chuanxiang Qin , Lixing Dai . Polyvinyl alcohol fiber with enhanced strength and modulus and intense cyan fluorescence based on covalently functionalized graphene quantum dots. Chinese Chemical Letters, 2025, 36(2): 110510-. doi: 10.1016/j.cclet.2024.110510
16. [16]
  Jingyu Chen , Sha Wu , Yuhao Wang , Jiong Zhou . Near-perfect separation of alicyclic ketones and alicyclic alcohols by nonporous adaptive crystals of perethylated pillar[5]arene and pillar[6]arene. Chinese Chemical Letters, 2025, 36(4): 110102-. doi: 10.1016/j.cclet.2024.110102
17. [17]
  Zheng Zhang , Lei Shi , Bin Wang , Jingyuan Qu , Xiaoling Wang , Tao Wang , Qitao Jiang , Wuhong Xue , Xiaohong Xu . Epitaxial growth of full-vdW α-In₂Se₃/MoS₂ heterostructures for all-in-one sensing and memory-computing artificial visual system. Chinese Chemical Letters, 2025, 36(3): 109687-. doi: 10.1016/j.cclet.2024.109687
18. [18]
  Brandon Bishop , Shaofeng Huang , Hongxuan Chen , Haijia Yu , Hai Long , Jingshi Shen , Wei Zhang . Artificial transmembrane channel constructed from shape-persistent covalent organic molecular cages capable of ion and small molecule transport. Chinese Chemical Letters, 2024, 35(11): 109966-. doi: 10.1016/j.cclet.2024.109966
19. [19]
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142