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Citation: Zhao Li, Hai-bin Sun, Cong-yi Li, Yong-lai Lu, Wang Qiao, Nan-ying Ning, Li-qun Zhang, Ming Tian. Dispersion and Filler Network Structure of Fibrillar Silicates in Elastomers[J]. Chinese Journal of Polymer Science, ;2016, 34(7): 858-872. doi: 10.1007/s10118-016-1801-9 shu

Dispersion and Filler Network Structure of Fibrillar Silicates in Elastomers

  • a.

    State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029, China

  • b.

    Aeolus Tyre Co., Ltd, Henan 454003, China

  • c.

    Office of Scientific Research and Development, Beijing University of Chemical Technology, Beijing 100029, China

  • d.

    PetroChina Sichuan Petrochemical Co. Ltd, Chengdu 611000, China

  • Corresponding author: Nan-ying Ning, ningny@mail.buct.edu.cn Ming Tian, tian71402@126.com
  • Received Date: 16 January 2016
    Revised Date: 19 February 2016
    Accepted Date: 28 February 2016

    Fund Project: This work was financially supported by the National Science Fund for Distinguished Young Scholars of China 51525301the National Basic Research Program of China 2015CB654704the National Natural Science Foundation of China 51373012

  • The dispersion and filler network of fibrillar silicate (FS) in elastomers were studied. The results showed that a good dispersion of FS in matrix during mechanical blending in unvulcanized composites contributed to a strong FS filler network, different from that of traditional reinforcing fillers. Meanwhile, the filler re-aggregation during vulcanization caused by the overlapping and intertwining of FS further strengthened the filler network. The factors including Mooney viscosity and molecular polarity of elastomer, type and amount of silane coupling agents used for filler modification, that may influence the filler network, were studied. Our study helps us to understand the mechanism for the formation of filler network of FS in elastomers and provides guidance for the preparation of high performance FS/elastomer composites.
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