Z-scheme基光电化学传感器的构建及其研究进展

引用本文: 杜凤峦, 赵春芹, 丁收年. Z-scheme基光电化学传感器的构建及其研究进展[J]. 分析化学, 2021, 49(8): 1247-1257. doi: 10.19756/j.issn.0253-3820.211135 shu

Citation: DU Feng-Luan, ZHAO Chun-Qin, DING Shou-Nian. Construction and Recent Progress of Z-scheme-based Photoelectrochemical Sensor[J]. Chinese Journal of Analytical Chemistry, 2021, 49(8): 1247-1257. doi: 10.19756/j.issn.0253-3820.211135 shu

Z-scheme基光电化学传感器的构建及其研究进展

东南大学化学化工学院, 南京 211189

通讯作者: 丁收年,E-mail:snding@seu.edu.cn

基金项目:
国家重点研发计划项目（No.2017YFA0700404）、国家自然科学基金项目（Nos.21535003，21575022）、江苏省重点研究发展计划项目（No.BE2018617）、中央高校基本科研业务费项目（No.2242016K41055）和江苏省研究生科研与实践创新计划项目（No.KYCX19_0073）资助。

摘要: 光活性半导体之间的电子转移路径对光电化学传感器的光电性能具有重要影响，有效的电子传输方式对增强光电转换效率和提升传感器的灵敏度均具有重要意义。Z-scheme机制在提升光致载流子迁移效率的同时，可最大程度地保留光电活性半导体的氧化还原能力。因此，Z-scheme基光电化学传感体系的构建和设计备受关注。本文以Z-scheme光电化学传感体系的电子转移机理及传感策略为主线，综述了Z-scheme基光电化学传感器的构建及研究进展。首先，总结了具有电子介体的Z-scheme系统和直接Z-scheme系统的这两条电子转移路径，提出了Z-scheme基PEC传感系统的结构；然后，将文献报道的Z-scheme系统的传感策略的设计系统地归纳为4个方面，包括空间位阻效应、引入新能级水平、靶抑制流子重组/迁移和靶诱导Z-scheme系统形成/改变；最后，对Z-scheme基光电化学传感器的发展前景进行了展望。

关键词:

English

Construction and Recent Progress of Z-scheme-based Photoelectrochemical Sensor

School of Chemistry and Chemical Engineering, Southeast University, Nanjing 211189, China

Corresponding author: DING Shou-Nian, snding@seu.edu.cn

Received Date: 22 February 2021
Revised Date: 07 May 2021
Fund Project:
Supported by the National Key Research and Development Program of China (No.2017YFA0700404), the National Natural Science Foundation of China (Nos.21535003, 21575022), the Key Research & Development Plan of Jiangsu Province (No.BE2018617), the Fundamental Research Funds for the Central Universities (No.2242016K41055) and the Postgraduate Research & Practice Innovation Program of Jiangsu Province (No.KYCX19_0073).

Abstract: The route of electron transfer between photoactive semiconductors has great impact on the photoelectric performance of photoelectrochemical (PEC) sensor. Thus, an effective electron transfer pathway is of great significance for enhancing the photoelectric conversion efficiency and improving the sensitivity of the sensor. Z-scheme mechanism can improve the migration efficiency of photogenerated carriers while retaining maximized redox capacity of the photoactive semiconductor. Therefore, the construction and design of the Z-scheme-based PEC sensing system has attracted the attention of many researchers. In this review, the construction and recent progress of Z-scheme-based PEC sensor are summarized in view of the electron transfer mechanism and sensing strategies. Firstly, we present the configuration of Z-scheme-based PEC sensor system by summarizing the two electron transfer paths of Z-scheme system with electronic mediator and direct Z-scheme system. Then, the as-reported sensing strategies regarding Z-scheme system are systematically summarized into four aspects, including steric resistance effect, introduction of new energy level, target inhibition of carrier recombination/migration, and target-induced of Z-scheme system formation/transformation. Finally, future outlooks toward Z-scheme PEC sensor are highlighted.

Key words:

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1.
沈阳化工大学材料科学与工程学院沈阳 110142

Z-scheme基光电化学传感器的构建及其研究进展

通讯作者: 丁收年,E-mail:snding@seu.edu.cn

English

Construction and Recent Progress of Z-scheme-based Photoelectrochemical Sensor

Corresponding author: DING Shou-Nian, snding@seu.edu.cn

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

计量

通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

Z-scheme基光电化学传感器的构建及其研究进展

通讯作者: 丁收年,E-mail:snding@seu.edu.cn

English

Construction and Recent Progress of Z-scheme-based Photoelectrochemical Sensor

Corresponding author: DING Shou-Nian, snding@seu.edu.cn

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

计量

文章相关

通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs