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PEG-VN改性PP隔膜用于高稳定性高效率锂硫电池

石英彤 ,  徐国桐 ,  梁贵增 ,  兰笛 ,  张思远 ,  王彦儒 ,  李道浩 ,  吴广磊

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引用本文: 石英彤, 徐国桐, 梁贵增, 兰笛, 张思远, 王彦儒, 李道浩, 吴广磊. PEG-VN改性PP隔膜用于高稳定性高效率锂硫电池[J]. 物理化学学报, 2025, 41(7): 100082. doi: 10.1016/j.actphy.2025.100082 shu
Citation:  Yingtong Shi, Guotong Xu, Guizeng Liang, Di Lan, Siyuan Zhang, Yanru Wang, Daohao Li, Guanglei Wu. PEG-VN改性PP隔膜用于高稳定性高效率锂硫电池[J]. Acta Physico-Chimica Sinica, 2025, 41(7): 100082. doi: 10.1016/j.actphy.2025.100082 shu

PEG-VN改性PP隔膜用于高稳定性高效率锂硫电池

  • 1.

    青岛大学材料科学与工程学院, 生物纤维与生态纺织国家重点实验室, 山东 青岛 266071

  • 2.

    青岛滨海学院新型金属功能材料青岛工程研究中心, 山东省高校先进金属功能材料及其加工特色实验室, 山东 青岛 266555

  • 3.

    湖北汽车工业学院汽车材料学院, 湖北 十堰 442002

  • 4.

    西北工业大学化学与化工学院, 陕西 西安 710072

    • 通讯作者: 王彦儒, yrwang1996@163.com; 李道浩, lidaohao@qdu.edu.cn; 吴广磊, wuguanglei@mail.xjtu.edu.cn
  • 基金项目:

    国家自然科学基金 52302272

    国家自然科学基金 52377026

    山东省泰山学者青年专家计划 tsqn202211124

    山东省泰山学者青年专家计划 tsqn202103057

    山东省自然科学基金 ZR2022QB023

    山东省自然科学基金 ZR2024ME046

    山东省高等学校青创人才引育计划“海洋多糖纤维基能源材料研究创新团队”及青岛大学生物纤维与生态纺织品国家重点实验室 ZKT10

    山东省高等学校青创人才引育计划“海洋多糖纤维基能源材料研究创新团队”及青岛大学生物纤维与生态纺织品国家重点实验室 GZRC202006

  • †These authors contributed equally to this work.
摘要: 锂硫(Li-S)电池因其高理论能量密度被视为下一代能源存储系统中最有前景的候选者之一。然而，Li-S电池的实际应用受到锂离子(Li+)传输效率低和由于穿梭效应引起的快速容量衰减的限制。在此，我们报道了一种复合材料，由聚乙二醇(PEG)和氮化钒(VN)纳米片涂覆在商业聚丙烯(PP)隔膜上，称为PEG-VN@PP隔膜。VN纳米片所表现出的超催化效应和吸附特性显著增强了多硫化物的转化，从而提高了Li-S电池的容量和稳定性。由于PEG的涂层，Li+被极性官能团吸引，实现了选择性传输，改善了Li+的传输效率和Li-S电池的倍率性能。使用硫质量负载为1.2 mg·cm−2的碳纳米管/硫阴极组装的Li-S电池，展现出高达782.0 mAh·g−1的比容量，并在1C (1675 mA·g−1)条件下经过700个循环后平均容量衰减为0.048%。

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  • 发布日期:  2025-07-15
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