钠离子电池阵列化负极材料的研究进展

引用本文: 陈瑶, 董浩洋, 李园园, 刘金平. 钠离子电池阵列化负极材料的研究进展[J]. 物理化学学报, 2021, 37(12): 200707. doi: 10.3866/PKU.WHXB202007075 shu

Citation: Yao Chen, Haoyang Dong, Yuanyuan Li, Jinping Liu. Recent Advances in 3D Array Anode Materials for Sodium-Ion Batteries[J]. Acta Physico-Chimica Sinica, 2021, 37(12): 200707. doi: 10.3866/PKU.WHXB202007075 shu

钠离子电池阵列化负极材料的研究进展

陈瑶 ^1, ,
董浩洋 ^1, ,
李园园 ^{2,
,} ,
刘金平 ^{1,
,}

1.
武汉理工大学化学化工与生命科学学院，材料复合新技术国家重点实验室，武汉 430070
2.
华中科技大学光学与电子信息学院，武汉 430074

作者简介:

李园园，华中科技大学光学与电子信息学院副教授，出生于1982年。2009年于华中师范大学获得博士学位，2018年在澳大利亚伍伦贡大学进行访学研究。当前主要研究方向为纳米结构材料的制备及其在电化学储能领域(超级电容器和电池)的应用;
刘金平，武汉理工大学首席教授，英国皇家化学学会会士(FRSC)，湖北黄冈人，出生于1981年。2009年在华中师范大学获得博士学位，2008-2011年期间先后在新加坡南洋理工大学(NTU)进行访问和博士后研究。现主要从事新能源材料与器件方面的研究(新型二次电池、超级电容器等);

通讯作者: 李园园, liyynano@hust.edu.cn; 刘金平, liujp@whut.edu.cn

基金项目:
国家自然科学基金 51972257

国家自然科学基金 51872104

国家自然科学基金 51672205

国家重点研发计划 2016YFA0202602

摘要: 钠离子电池具有钠资源储量丰富、成本低以及安全系数高等优点，在大规模储能、新能源汽车和柔性/可穿戴电子领域中显示出巨大的潜力。然而，钠离子较大的离子半径会造成电极电化学反应动力学缓慢、材料体积变化大等问题，因此开发有利于钠离子嵌入/脱出、稳定性强和容量高的电极材料至关重要。相比于传统的粉末涂覆电极，无粘结剂的三维阵列电极在形成连续的电子传输通道、促进电解液渗透和缩短离子扩散路径等方面更具优势。本文综述了单质、过渡金属氧化物、硫化物、磷化物和钛酸盐等阵列负极材料在钠离子电池中的最新研究进展。重点介绍了各类阵列负极的制备方法、结构/形貌特点和储钠性能，最后对钠离子电池阵列化电极未来的机遇和挑战进行了展望。

关键词:

English

Recent Advances in 3D Array Anode Materials for Sodium-Ion Batteries

Yao Chen ^1, ,
Haoyang Dong ^1, ,
Yuanyuan Li ^{2,
,} ,
Jinping Liu ^{1,
,}

1.
School of Chemistry, Chemical Engineering and Life Science, State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China
2.
School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, China

Corresponding author: Email: liyynano@hust.edu.cn (Y.L.); Email: liujp@whut.edu.cn (J.L.)

Received Date: 26 July 2020
Accepted Date: 18 August 2020
Revised Date: 18 August 2020
Available Online: 15 December 2021
Fund Project:
the National Natural Science Foundation of China

the National Natural Science Foundation of China

the National Natural Science Foundation of China

the National Key R&D Program of China

Abstract: Lithium-ion batteries have achieved tremendous success in the fields of portable mobile devices, electric vehicles, and large-scale energy storage owing to their high working voltage, high energy density, and long-term lifespan. However, lithium-ion batteries are ultimately unable to satisfy increasing industrial demands due to the shortage and rising cost of lithium resources. Sodium is another alkali metal that has similar physical and chemical properties to those of lithium, but is more abundant. Therefore, sodium-ion batteries (SIBs) are promising candidates for next-generation energy storage devices. Nevertheless, SIBs generally exhibit inferior electrochemical reaction kinetics, cycling performance, and energy density to those of lithium-ion batteries owing to the larger ion radius and higher standard potential of Na+ compared to those of Li+. To address these issues, significant effort has been made toward developing electrode materials with large sodiation/desodiation channels, robust structural stability, and high theoretical capacity. As electrode performance is closely related to its architecture, constructing an advanced electrode structure is crucial for achieving high-performance SIBs. Conventional electrodes are generally prepared by mixing a slurry of active materials, conductive carbon, and binders, followed by casting on a metal current collector. Electrodes prepared this way are subject to shape deformation, causing the active materials to easily peel off the current collector during charge/discharge processes. This leads to rapid capacity decay and short cycle life. Moreover, binders and other additives increase the weight and volume of the electrodes, which reduces the overall energy density of the batteries. Therefore, binder-free, three-dimensional (3D) array electrodes with satisfactory electronic conductivity and low ion-path tortuosity have been proposed. In addition to solving the aforementioned issues, this type of electrode significantly reduces contact resistance through the strong adhesion between the array and the substrate. Furthermore, electrolyte infiltration is greatly facilitated by the abundant interspacing between individual nanostructures, which promotes fast electron transport and shortens ion diffusion, thus enabling the electrode reaction. The array structure can also readily accommodate substantial volume variations that occur during repeated sodiation/desodiation processes and release the generated stress. Therefore, it is of great interest to explore binder-free array electrodes for sodium-ion storage applications. This review summarizes the recent advances in various 3D array anode materials for SIBs, including elemental anodes, transition metal oxides, sulfides, phosphides, and titanates. The preparation methods, structure/morphology characteristics, and electrochemical performance of various array anodes are discussed, and future opportunities and challenges from employing array electrodes in SIBs are proposed.

Key words:

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沈阳化工大学材料科学与工程学院沈阳 110142

钠离子电池阵列化负极材料的研究进展

通讯作者: 李园园, liyynano@hust.edu.cn; 刘金平, liujp@whut.edu.cn

English

Recent Advances in 3D Array Anode Materials for Sodium-Ion Batteries

Corresponding author: Email: liyynano@hust.edu.cn (Y.L.); Email: liujp@whut.edu.cn (J.L.)

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通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

钠离子电池阵列化负极材料的研究进展

通讯作者: 李园园, liyynano@hust.edu.cn; 刘金平, liujp@whut.edu.cn

English

Recent Advances in 3D Array Anode Materials for Sodium-Ion Batteries

Corresponding author: Email: liyynano@hust.edu.cn (Y.L.); Email: liujp@whut.edu.cn (J.L.)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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