Citation: LIU Feng-Xian, SHAO Meng-Meng, XIA Sheng-Jie, NI Zhe-Ming. Adsorption to Acid Red 14 in Wastewater by ZnCr Bimetal Layered Materials[J]. Chinese Journal of Inorganic Chemistry, ;2015, 31(7): 1342-1350. doi: 10.11862/CJIC.2015.187 shu

Adsorption to Acid Red 14 in Wastewater by ZnCr Bimetal Layered Materials

1.
College of Chemical Engineering, Zhejiang University of Technology, Hangzhou 310014, China

Corresponding author: NI Zhe-Ming,
Received Date: 1 February 2015
Available Online: 13 May 2015
Fund Project: 浙江省自然科学基金(No.LQ15B030002)资助项目。 (No.LQ15B030002)

Zinc chrome bimetal layered materials (Zn_xCr-LDHs, x=2, 3, 4) were successfully synthesized by the coprecipitation method and different factors on the adsorption of AR14 were also investigated. The characterization of XRD, ICP, FTIR and BET revealed that the crystal structures of Zn_xCr-LDHs (x=2, 3, 4) were very good and stable, it had the mesoporous structure. Experimental results indicated that the optimum sorbent was Zn₃Cr-LDHs with a specific surface area of 101 m²·g^-1, the maximum adsorption capacity for AR14 was 484.63 mg·g^-1. Moreover, lower pH value and higher temperature were favorable to the removal of AR14. Adsorption isotherms and kinetics showed that the adsorption process could be well fitted with the pseudo-second-order kinetic and Freundlich equation. Based on the analysis of Materials Studio 5.5 simulation, the adsorption menchanism was that AR14 were adsorbed on the surface of Zn₃Cr-LDHs, the -SO₃^- group was the reaction point.
- ZnCr layered double hydroxides;adsorption;acid red 14
1. [1]
  [1] Gao J F, Wang J H, Yang C, et al. Chem. Eng. J., 2011, 171 (3):967-975
2. [2]
  [2] Wang S, Choon W N, Wang W, et al. Chem. Eng. J., 2012, 197:34-40
3. [3]
  [3] Arami M, Limaee N Y, Mahmoodi N M, et al. J. Hazard. Mater., 2006, 135(1/2/3):171-179
4. [4]
  [4] Arami M, Limaee N Y, Mahmoodi N M. Chem. Eng. J., 2008, 139(1):2-10
5. [5]
  [5] Valderrama C, Cortina J L, Farran A, et al. React. Funct. Polym., 2008, 68(3):679-691
6. [6]
  [6] CHEN Shu-Wei(陈树薇), SHI Wen-Jian(施文健), SONG Wei(宋伟), et al. J. Funct. Mater.(功能材料), 2009, 40(4): 656-659
7. [7]
  [7] Mahmoodi N M, Khorramfar S, Najafi F. Desalination, 2011, 279(1/2/3):61-68
8. [8]
  [8] Mahmoodi N M, Najafi F. Microporous Mesoporous Mater., 2012, 156:153-160
9. [9]
  [9] Mahmoodi N M, Masrouri O, Arabi A M. J. Alloys Compd., 2014, 602:210-220
10. [10]
  [10] Gennequin C, Barakat T, Tidahy H L, et al. Catal. Today, 2010, 157(1/2/3/4):191-197
11. [11]
  [11] Zhang C, Yang S G, Chen H Z, et al. Appl. Surf. Sci., 2014, 301:329-337
12. [12]
  [12] Jimenez-Nunez M L, Solache-Rios M, Chavez-Garduno J, et al. Chem. Eng. J., 2012, 181:371-375
13. [13]
  [13] Zhou J B, Cheng Y, Yu J G, et al. J. Mater. Chem., 2011, 21 (48):19353-19361
14. [14]
  [14] Yang K, Yan L G, Yang Y M, et al. Sep. Purif. Technol., 2014, 124:36-42
15. [15]
  [15] Ni Z M, Xia S J, Wang L G, et al. J. Colloid Interface Sci., 2007, 316(2):284-291
16. [16]
  [16] XUE Ji-Long(薛继龙), CAO Gen-Ting(曹根庭), NI Zhe-Ming(倪哲明). Chinese J. Inorg. Chem.(无机化学学报), 2012, 28(6):1117-1124
17. [17]
  [17] WANG Qiao-Qiao(王巧巧), NI Zhe-Ming(倪哲明), ZHANG Feng(张峰), et al. Chinese J. Inorg. Chem.(无机化学学报), 2009, 25(12):2156-2162
18. [18]
  [18] XUE Ji-Long(薛继龙), QIAN Ping-Ping(钱萍萍), NI Zhe-Ming(倪哲明). Chinese J. Inorg. Chem.(无机化学学报), 2014, 30(5):1009-1016
19. [19]
  [19] Gasser M S, Aly H F. Colloid Surf. A-Physicochem. Eng. Asp., 2009, 336(1/2/3):167-173
20. [20]
  [20] Zhou Z J, Wu Y Y, Liu C, et al. Environ. Sci. Technol., 2010, 44(23):8884-8890
21. [21]
  [21] Parida K, Mohapatra L. Dalton Trans., 2012, 41:1173-1178
22. [22]
  [22] Gunjakar J L, Kim T W, Kim H N, et al. J. Am. Chem. Soc., 2011, 133(38):14998-15007
23. [23]
  [23] Chen D, Li Y, Zhang J, et al. Chem. Eng. J., 2012, 185:120-126
24. [24]
  [24] Lan M, Fan G L, Yang L, et al. Ind. Eng. Chem. Res., 2014, 53:12943-12952
25. [25]
  [25] WANG Xiao-Rong(王小蓉), WU Ping-Xiao(吴平霄). Environ. Sci.(环境科学), 2012, 33(7):2432-2437
26. [26]
  [26] GU Jian-Jie(顾剑杰), WANG Yan-Feng(王炎锋), JIANG Ru (蒋茹), et al. Ind. Water & Wastewater(工业用水与废水), 2014, 45(2):9-13
27. [27]
  [27] Xia S J, Liu F X, Ni Z M, et al. J. Colloid Interface Sci., 2013, 405:195-200
28. [28]
  [28] Jiao F P, Chen X Q, Liu L, et al. J. Mol. Struct., 2010, 964 (1/2/3):152-157
29. [29]
  [29] Ai L H, Zhang C Y, Meng L Y. J. Chem. Eng. Data, 2011, 56(11):4217-4225
1. [1]
  Jingke LIU , Jia CHEN , Yingchao HAN . Nano hydroxyapatite stable suspension system: Preparation and cobalt adsorption performance. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1763-1774. doi: 10.11862/CJIC.20240060
2. [2]
  Peng XU , Shasha WANG , Nannan CHEN , Ao WANG , Dongmei YU . Preparation of three-layer magnetic composite Fe₃O₄@polyacrylic acid@ZiF-8 for efficient removal of malachite green in water. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 544-554. doi: 10.11862/CJIC.20230239
3. [3]
  Zeyu XU , Anlei DANG , Bihua DENG , Xiaoxin ZUO , Yu LU , Ping YANG , Wenzhu YIN . Evaluation of the efficacy of graphene oxide quantum dots as an ovalbumin delivery platform and adjuvant for immune enhancement. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1065-1078. doi: 10.11862/CJIC.20240099
4. [4]
  Shuanglin TIAN , Tinghong GAO , Yutao LIU , Qian CHEN , Quan XIE , Qingquan XIAO , Yongchao LIANG . First-principles study of adsorption of Cl₂ and CO gas molecules by transition metal-doped g-GaN. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1189-1200. doi: 10.11862/CJIC.20230482
5. [5]
  Chuanming GUO , Kaiyang ZHANG , Yun WU , Rui YAO , Qiang ZHAO , Jinping LI , Guang LIU . Performance of MnO₂-0.39IrO_x composite oxides for water oxidation reaction in acidic media. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1135-1142. doi: 10.11862/CJIC.20230459
6. [6]
  Xiaosong PU , Hangkai WU , Taohong LI , Huijuan LI , Shouqing LIU , Yuanbo HUANG , Xuemei LI . Adsorption performance and removal mechanism of Cd(Ⅱ) in water by magnesium modified carbon foam. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1537-1548. doi: 10.11862/CJIC.20240030
7. [7]
  Jie ZHAO , Sen LIU , Qikang YIN , Xiaoqing LU , Zhaojie WANG . Theoretical calculation of selective adsorption and separation of CO₂ by alkali metal modified naphthalene/naphthalenediyne. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 515-522. doi: 10.11862/CJIC.20230385
8. [8]
  Youlin SI , Shuquan SUN , Junsong YANG , Zijun BIE , Yan CHEN , Li LUO . Synthesis and adsorption properties of Zn(Ⅱ) metal-organic framework based on 3, 3', 5, 5'-tetraimidazolyl biphenyl ligands. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1755-1762. doi: 10.11862/CJIC.20240061
9. [9]
  Xinyu Yin , Haiyang Shi , Yu Wang , Xuefei Wang , Ping Wang , Huogen Yu . Spontaneously Improved Adsorption of H₂O and Its Intermediates on Electron-Deficient Mn^(3+δ)+ for Efficient Photocatalytic H₂O₂ Production. Acta Physico-Chimica Sinica, 2024, 40(10): 2312007-. doi: 10.3866/PKU.WHXB202312007
10. [10]
  Xin Lu , Haoran Sun , Xiaomeng Li , Chunrui Li , Jinfeng Wang , Dandan Zhou . C14-HSL limits the mycelial morphology of pathogen Trichosporon cells but enhances their aggregation: Mechanisms and implications. Chinese Chemical Letters, 2024, 35(6): 108936-. doi: 10.1016/j.cclet.2023.108936
11. [11]
  Jingping Hu , Jing Xu . Total synthesis of a putative yuzurimine-type Daphniphyllum alkaloid C₁₄–epi-deoxycalyciphylline H. Chinese Chemical Letters, 2024, 35(4): 108733-. doi: 10.1016/j.cclet.2023.108733
12. [12]
  Xingyang LI , Tianju LIU , Yang GAO , Dandan ZHANG , Yong ZHOU , Meng PAN . A superior methanol-to-propylene catalyst: Construction via synergistic regulation of pore structure and acidic property of high-silica ZSM-5 zeolite. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1279-1289. doi: 10.11862/CJIC.20240026
13. [13]
  Kai CHEN , Fengshun WU , Shun XIAO , Jinbao ZHANG , Lihua ZHU . PtRu/nitrogen-doped carbon for electrocatalytic methanol oxidation and hydrogen evolution by water electrolysis. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1357-1367. doi: 10.11862/CJIC.20230350
14. [14]
  Wen YANG , Didi WANG , Ziyi HUANG , Yaping ZHOU , Yanyan FENG . La promoted hydrotalcite derived Ni-based catalysts: In situ preparation and CO₂ methanation performance. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 561-570. doi: 10.11862/CJIC.20230276
15. [15]
  Doudou Qin , Junyang Ding , Chu Liang , Qian Liu , Ligang Feng , Yang Luo , Guangzhi Hu , Jun Luo , Xijun Liu . Addressing Challenges and Enhancing Performance of Manganese-based Cathode Materials in Aqueous Zinc-Ion Batteries. Acta Physico-Chimica Sinica, 2024, 40(10): 2310034-. doi: 10.3866/PKU.WHXB202310034
16. [16]
  Xiaoning TANG , Junnan LIU , Xingfu YANG , Jie LEI , Qiuyang LUO , Shu XIA , An XUE . Effect of sodium alginate-sodium carboxymethylcellulose gel layer on the stability of Zn anodes. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1452-1460. doi: 10.11862/CJIC.20240191
17. [17]
  Xiaoning TANG , Shu XIA , Jie LEI , Xingfu YANG , Qiuyang LUO , Junnan LIU , An XUE . Fluorine-doped MnO₂ with oxygen vacancy for stabilizing Zn-ion batteries. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1671-1678. doi: 10.11862/CJIC.20240149
18. [18]
  Lu XU , Chengyu ZHANG , Wenjuan JI , Haiying YANG , Yunlong FU . Zinc metal-organic framework with high-density free carboxyl oxygen functionalized pore walls for targeted electrochemical sensing of paracetamol. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 907-918. doi: 10.11862/CJIC.20230431
19. [19]
  Qiuyang LUO , Xiaoning TANG , Shu XIA , Junnan LIU , Xingfu YANG , Jie LEI . Application of a densely hydrophobic copper metal layer in-situ prepared with organic solvents for protecting zinc anodes. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1243-1253. doi: 10.11862/CJIC.20240110

Get Citation

PDF

XML

Metrics

PDF Downloads(0)
Abstract views(199)
HTML views(26)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142